Surface science studies of electrochemical energy storage de

Carbon Materials with Hierarchical Pore Structure for Electrochemical Energy Storage Devices
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We also discuss the application of 3D porous architectures as conductive scaffolds for various electrode materials to enable composite electrodes with an unprecedented combination of energy and power densities and then conclude with a perspective on future opportunities and challenges. Kang, K. Electrodes with high power and high capacity for rechargeable lithium batteries. Science , — Chiang, Y. Building a better battery.

Simon, P. Materials for electrochemical capacitors. Arico, A. Nanostructured materials for advanced energy conversion and storage devices. Anasori, B. Lin, M. An ultrafast rechargeable aluminium-ion battery. Nature , — This study reports an ultrafast-charging aluminium battery composed of a 3D graphitic foam cathode, which offers a safe alternative to commercial Li-ion batteries.

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Electrochemical surface science (EC-SS) is the natural advancement of traditional surface science (where gas-vacuum/solid interfaces are studied) to need for a rational design of energy conversion and storage devices for next generation. an Electrolyte Additive to Modify Electrode Surface and Suppress Dissolution of Polysulfides The subjects will range from fundamental studies of electrode processes, their flow batteries, and their components,; electrochemical materials science. This journal covers all aspects of electrochemical energy storage and.

Augustyn, V. Bruce, P. Li—O 2 and Li—S batteries with high energy storage. Sun, H. This study reports a 3D HG scaffold supporting high-performance electrode materials, forming a composite that is capable of efficient charge delivery even at high areal mass loading. Liu, J. Charging graphene for energy. Where do batteries end and supercapacitors begin? Tarascon, J. Issues and challenges facing rechargeable lithium batteries.

Raccichini, R. The role of graphene for electrochemical energy storage. This progress article outlines the most promising results and applications of graphene for electrochemical energy storage. An, Q. Three-dimensional porous V 2 O 5 hierarchical octahedrons with adjustable pore architectures for long-life lithium batteries. Nano Res. High-rate lithiation-induced reactivation of mesoporous hollow spheres for long-lived lithium-ion batteries.

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Zhang, N. Spherical nano-Sb C composite as a high-rate and ultra-stable anode material for sodium-ion batteries. Li, L. Graphene-wrapped MnO 2 —graphene nanoribbons as anode materials for high-performance lithium ion batteries. Xu, J. Nitrogen-doped holey graphene as an anode for lithium-ion batteries with high volumetric energy density and long cycle life. Small 11 , — Wu, R. ACS Nano 8 , — Xia, Y. Thickness-independent capacitance of vertically aligned liquid-crystalline MXenes.

Lukatskaya, M. Ultra-high-rate pseudocapacitive energy storage in two-dimensional transition metal carbides. Energy 2 , Wang, M. Reversible calcium alloying enables a practical room-temperature rechargeable calcium-ion battery with a high discharge voltage. Qie, L. Highly rechargeable lithium-CO 2 batteries with a boron- and nitrogen-codoped holey-graphene cathode. Dudney, N. Using all energy in a battery. Graphene-wrapped mesoporous cobalt oxide hollow spheres anode for high-rate and long-life lithium ion batteries.

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C , — Liu, N. A pomegranate-inspired nanoscale design for large-volume-change lithium battery anodes. Wu, H. Stable cycling of double-walled silicon nanotube battery anodes through solid-electrolyte interphase control. Lim, E. Facile synthesis of Nb 2 O 5 carbon core—shell nanocrystals with controlled crystalline structure for high-power anodes in hybrid supercapacitors.

ACS Nano 9 , — Wang, G. Nano Energy 36 , 46—57 Zhong, Y. Simultaneously armored and active graphene for transparent and flexible supercapacitors. Wang, H. Ni OH 2 nanoplates grown on graphene as advanced electrochemical pseudocapacitor materials. Li, Y. Growth of conformal graphene cages on micrometre-sized silicon particles as stable battery anodes. Energy 1 , Cheng, H. Charge delivery goes the distance. Gogotsi, Y. True performance metrics in electrochemical energy storage. This perspective emphasizes the importance of true performance metrics to evaluate electrochemical performance when considering the inactive passive components in a practical device.

Gallagher, K. Optimizing areal capacities through understanding the limitations of lithium-ion electrodes. This study demonstrates the importance of the mass transport limit of ions in thick electrodes and defines a penetration depth to study the utilization of the active materials at a high level of mass loading.

Fang, R. Singh, M. Thick electrodes for high energy lithium ion batteries. Moshtev, R. State of the art of commercial Li ion batteries. Power Sources 91 , 86—91 Zhu, H. Tin anode for sodium-ion batteries using natural wood fiber as a mechanical buffer and electrolyte reservoir. Nano Lett. Zhu, M. Highly anisotropic, highly transparent wood composites. Yao, H. Crab shells as sustainable templates from nature for nanostructured battery electrodes. Hyde, S. Geometry of interfaces: topological complexity in biology and materials.

Interface Focus 2 , — Zhu, J. A hyperaccumulation pathway to three-dimensional hierarchical porous nanocomposites for highly robust high-power electrodes. Werner, J. Block copolymer derived 3D interpenetrating multifunctional gyroidal nanohybrids for electrical energy storage. Energy Environ. A bottom-up, block copolymer approach that enables the integration and interpenetration of many functional nanomaterials into 3D batteries, resulting in a substantial decrease in footprint area and improved performance compared with 2D designs.

Peng, H. Liu, W. Zhou, G. More reliable lithium — sulfur batteries: status, solutions and prospects. Cheng, X. Power Sources , — Zhao, S. A 3D multifunctional architecture for lithium—sulfur batteries with high areal capacity.

2019 Van Horn Distinguished Lectures: 1: electrochemical energy storage

Small 2 , High-performance sodium ion batteries based on a 3D anode from nitrogen-doped graphene foams. Hu, L. Silicon—carbon nanotube coaxial sponge as Li-ion anodes with high areal capacity. Energy Mater. Chen, Y. Densification by compaction as an effective low-cost method to attain a high areal lithium storage capacity in a CNT Co 3 O 4 sponge. Luo, B. Nanoscale 7 , — The cathodic peaks from a Pd-O region from 0.

RHE Fig. LSV and CA measurements in 0. The current density was normalized by the catalyst Pd loadings Figs. It is worth noting that specific current densities in Fig. At a potential of 0. To compare the steady-state activity at 0. RHE for one hour performed in 0. The C 2 product peaks started being detected at the potential of 0. Therefore, consistent with the DFT and surface science conclusions, the Pd-modified WC catalyst bound to the reaction intermediates more weakly, potentially resulting in less catalyst poisoning by the EOR intermediates.

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Overall, results presented in this study demonstrated the feasibility of designing EOR catalysts from fundamental DFT and surface science studies. DOE under Contract No. Jingguang G.

Chen This is an open access article distributed under the terms of the Creative Commons Attribution 4. User Name Password Sign In. Previous Section Next Section.

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Electrochemical measurements and stability test Electrochemical measurements were performed at room temperature in an alkaline 0. View this table: In this window In a new window. Table I. Figure 1. Figure 2. Table II. Table III. Figure 3. Figure 4. Figure 5. Figure 6. Table IV. Previous Section.

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Chemistry Division. Our Research We focus our research on both fundamental and applied problems relating to electrochemical energy storage systems and materials.